How heteroatoms influence the cross-conjugation and its impact on DSSC
Linear vs. Cross-conjugated Anchoring group
(Sprache: Englisch)
This book describs the unusual bonding pattern and proximal heteroatom substitution in p-cross conjugation produced distinct changes in the energy levels and photophysical behaviour of the dyes. To seek an understanding of the origin of these fluctuations,...
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This book describs the unusual bonding pattern and proximal heteroatom substitution in p-cross conjugation produced distinct changes in the energy levels and photophysical behaviour of the dyes. To seek an understanding of the origin of these fluctuations, we have carried out a detailed computational investigation on a series of D-p1-p2 (A1)-A2 structured dyes comprised of common donor-spacer (auxiliary acceptor) units but varied the anchoring parts. In this study, we introduced a novel dimethylamino substituted fluorene-based triarylamine donor unit and evaluated its donating strength. Based on the comparison of DFT computed energy levels with experimental results, we have proposed an orbital splitting pattern to explain the energy level and photophysical properties of the linear vs. cross-conjugated dyes with respect to the linking position of the anchoring unit and benzo[1,2,5]thiadiazole (BTD) substitution.
Autoren-Porträt von Mahalingavelar Paramasivam
Paramasivam, MahalingavelarM. Paramasivam has obtained his PhD from CSIR-IICT, Hyderabad, India; His research interests are development of novel organic molecules for DSSCs, PeSCs, BHJSCs, TADF Emitters, OFETs, AIE materials, Organic Photocatalysts and COFs.
Bibliographische Angaben
- Autor: Mahalingavelar Paramasivam
- 2018, 88 Seiten, Maße: 22 cm, Kartoniert (TB), Englisch
- Verlag: Scholar's Press
- ISBN-10: 363971735X
- ISBN-13: 9783639717358
Sprache:
Englisch
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