Supported Ionic Liquids
Fundamentals and Applications
(Sprache: Englisch)
Gives a timely overview about the fundamentals and applications of supported ionic liquids in modern organic synthesis
Introduces the concept and synthesis of supported ionic liquid phase (SILP) materials
Presents important applications in the field of catalysis (e.g.
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Produktinformationen zu „Supported Ionic Liquids “
Gives a timely overview about the fundamentals and applications of supported ionic liquids in modern organic synthesis
Introduces the concept and synthesis of supported ionic liquid phase (SILP) materials
Presents important applications in the field of catalysis (e.g.
Klappentext zu „Supported Ionic Liquids “
Technology with supported ionic liquids is a fundamental new approach to modifying the surfaces of porous solids by dispersing a thin film of ionic liquid onto it. The technology allows introducing new and unique material properties and attains long-term stable materials. Divided into four parts, this book introduces the topic of supported ionic liquid materials and fundamentals, covering ionic liquids, porous supports, synthesis and characterization. The main part covers various applications, such as the catalytic production of bulk and fine chemicals, environmental processes, biotechnology, energy production and gas separation. In each case, the most pertinent authors available describe here the underlying research. The final part discusses the perspectives and outlook of these materials as well as describing some real life applications.This book is aimed at organic and inorganic chemists, industrial chemists, catalytic chemists, chemical engineers, biotechnologists, materials scientists and libraries
Inhaltsverzeichnis zu „Supported Ionic Liquids “
PrefaceINTRODUCTIONA Century of Supported LiquidsSupported Ionic LiquidsApplications in CatalysisApplications in SeparationCoating of Heerogeneous CatalystsMonolayers of IL on SurfacesConclusionPART I: Concept and Building BlocksINTRODUCING IONIC LIQUIDSIntroductionPreparationLiquid RangeStructuresPhysical PropertiesEffects of Ionic Liquids on Chemical ReactionsIonic Liquids as Process Solvents in IndustrySummaryPOROUS INORGANIC MATERIALS AS POTENTIAL SUPPORTS FOR IONIC LIQUIDSIntroductionPorous Materials - An OverviewSilica-Based Materials - AmorphousLayered MaterialsOrdered Mesoporous MaterialsStructured Supports and Monolithic MaterialsConclusionsSYNTHETIC METHODOLOGIES FOR SUPPORTED IONIC LIQUID MATERIALSIntroductionSupport MaterialsPreparation Methods for Supported Ionic LiquidsSummaryPART II: Synthesis and PropertiesPORE VOLUME AND SURFACE AREA OF SUPPORTED IONIC LIQUIDS SYSTEMSExample I: [EMIM][NTf2] on Porous SilicaExample II: SCILL Catalyst (Commercial Ni catalyst) Coated with [BMIM][OcSO4]TRANSPORT PHENOMENA, EVAPORATION, AND THERMAL STABILITY OF SUPPORTED IONIC LIQUIDSIntroductionDiffusion of Gases and Liquids in ILs and Diffusivity of ILs in GasesThermal Stability and Vapor Pressure of Pure ILsVapor Pressure and Thermal Decomposition of Supported ILsOutlookIONIC LIQUIDS AT THE GAS-LIQUID AND SOLID-LIQUID INTERFACE - CHARACTERIZATION AND PROPERTIESIntroductionCharacterization of Ionic Liquid Surfaces by Spectroscopic TechniquesOrientation and Properties of Ionic Liquids at the Solid-Liquid InterfaceCommentsSPECTROSCOPY ON SUPPORTED IONIC LIQUIDSNMR-SpectroscopyIR SpectroscopyA PRIORI SELECTION OF THE TYPE OF IONIC LIQUIDIntroduction and ObjectiveMethodsUsage of COSMO-RS to Predict Solubilities in ILResults of Reaction ModelingPerspectives of the A Priori Selection of ILsPART III: Catalytic ApplicationsSUPPORTED IONIC LIQUIDS AS PART OF A BUILDING-BLOCK SYSTEM FOR TAILORED CATALYSTSIntroductionImmobilized CatalystsSupported Ionic LiquidsThe Building
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BlocksCatalysis in Supported Thin Films of ILSupported Films of IL in CatalysisAdvantages and Drawbacks of the ConceptConclusionsCOUPLING REACTIONS WITH SUPPORTED IONIC LIQUID CATALYSTSIntroductionA Short History of Supported Ionic LiquidsProperties of SILApplication of SIL in Coupling ReactionsConclusionSELECTIVE HYDROGENATION FOR FINE CHEMICAL SYNTHESISIntroductionSelective Hydrogenation of Alpha,Beta-Unsaturated AldehydesAsymmetric Hydrogenations over Chiral Metal Complexes Immobilize3d in SILCAsConclusionsHYDROGENATION WITH NANOPARTICLES USING SUPPORTED IONIC LIQUIDSIntroductionMNPs Dispersed in ILs: Green Catalysts for Multiphase ReactionsMNPs Immobilized on Supported Ionic Liquids: Alternative Materials for Catalytic ReactionsConclusionsSOLID CATALYSTS WITH IONIC LIQUID LAYER (SCILL)IntroductionClassification of Applications of Ionic Liquids in Heterogeneous CatalysisPreparation and Characterization of the Physical Properties of the SCILL SystemsKinetic Studies with SCILL CatalystsConclusions and OutlookSUPPORTED IONIC LIQUID PHASE (SILP) MATERIALS IN HYDROFORMYLATION CATALYSISSILP Materials in Liquid-Phase Hydroformylation ReactionsGas-Phase SILP Hydroformylation CatalysisSILP Combined with scCO2 - Extending the Substrate RangeContinuous SILP Gas-Phase Methanol CarbonylationConclusion and Future PotentialULTRALOW TEMPERATURE WATER-GAS SHIFT REACTION ENABLED BY SUPPORTED IONIC LIQUID PHASE CATALYSTSIntroduction to Water-Gas Shift ReactionChallengesSILP Catalyst DevelopmentBuilding-Block OptimizationApplication-Specific TestingConclusionBIOCATALYTIC PROCESSES BASED ON SUPPORTED IONIC LIQUIDSIntroduction and General ConceptsBiocatalysts Based on Supported Ionic Liquid Phases (SILPs)Biocatalysts Based on Covalently Supported Ionic Liquid-Like Phases (SILLPs)Conclusions/Future Trends and PerspectivesSUPPORTED IONIC LIQUID PHASE CATALYSTS WITH SUPERCRITICAL FLUID FLOWIntroductionSILP CatalysisPART IV: Special ApplicationsPHARMACEUTICALLY ACTIVE SUPPORTED IONIC LIQUIDSActive Pharmaceutical Ingredients in Ionic Liquid FormSolid-Supported PharmaceuticalsSilica Materials for Drug DeliveryFactors That Influence the Loading and Release Rate of DrugsSILPs Approach for Drug DeliveryConclusionsSUPPORTED PROTIC IONIC LIQUIDS IN POLYMER MEMBRANES FOR ELECTROLYTES OF NONHUMIDIFIED FUEL CELLSIntroductionProtic ILs as Electrolytes for Fuel CellsMembrane Fabrication Including PIL and Fuel Cell OperationProton Conducting Mechanism during Fuel Cell OperationConclusionGAS SEPARATION USING SUPPORTED IONIC LIQUIDSSILP MaterialsSupported Ionic Liquid Membranes (SILMs)ConclusionIONIC LIQUIDS ON SURFACES - A PLETHORA OF APPLICATIONSIntroductionThe Influence of ILs on Solid-State SurfacesLayers of ILs on Solid-State SurfacesSelected ApplicationsSensorsElectrochemical Double Layer Capacitors (Supercapacitors)Dye Sensitized Solar CellsLubricantsSynthesis and Dispersions of NanoparticlesPART V: OutlookOUTLOOK - THE TECHNICAL PROSPECT OF SUPPORTED IONIC LIQUID MATERIALSCompetitive AdvantageObservabilityTrialabilityCompatibilityComplexityPerceived Risk
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Autoren-Porträt
Rasmus Fehrmann is Professor and head of the Centre for Catalysis and Sustainable Chemistry at the Department of Chemistry, Technical University of Denmark (DTU). After obtaining his PhD from DTU he was awarded university candidate- and senior scholarships as well as postdoctoral fellowships at the Institute of Catalysis in Novosibirsk (Russia), Université de Provence (France), and University of Patras (Greece), before taking up his present appointment. His main scientific achievements fall within the chemistry of sulfuric acid catalysts, environmental catalysis and ionic liquid fundamentals and applications including SLP and SILP technologies. Professor Fehrmann has authored over 130 scientific publications, 20 patent applications, and 400 oral or poster presentations at international conferences, and has been a board member of the Danish National Committee for Chemistry for over a decade.Anders Riisager is Associate Professor at the Centre for Catalysis and Sustainable Chemistry at the Department of Chemistry, Technical University of Denmark (DTU). He studied Chemistry at the University of Copenhagen (Denmark) and obtained his PhD in catalysis from DTU in 2002. Subsequently he acquired a three-year postdoctoral fellowship at RWTH-Aachen/ University of Erlangen-Nuremberg (Germany) followed by a one-year Villum Kann Rasmussen postdoctoral fellowship at DTU, where he developed novel SILP catalysts and processes. He has authored more than 80 scientific publications and 20 patent applications, and received several honors including a nomination for the Degussa European Science-to-Business Award 2006 for SILP materials. His main scientific focus is the development of sustainable ionic liquid catalysis and separation technology.Marco Haumann has been a lecturer at the University of Erlangen-Nuremberg (FAU, Germany) since 2003. He studied Engineering and Chemistry at the universities of Dortmund and Berlin (Germany). After obtaining his PhD in 2001, he spent two years at
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the universities of Cape Town and Johannesburg (South Africa), developing novel catalysts in collaboration with Sasol Technology Pty Limited. From 2011 to the end of 2012, he was in charge of the establishment of the new FAU Branch Campus in Busan, South Korea. He has authored more than 40 scientific publications and was awarded the Arnold-Eucken prize of the Association of German Engineers (VDI-GVC) in 2011 for his contributions on SILP technology. His main scientific focus is the development of novel supported ionic liquid phase materials for catalysis and separation science.
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Bibliographische Angaben
- 2014, 496 Seiten, 30 farbige Abbildungen, 300 Schwarz-Weiß-Abbildungen, Maße: 17,2 x 25,1 cm, Gebunden, Englisch
- Herausgegeben: Rasmus Fehrmann, Anders Riisager, Marco Haumann
- Verlag: Wiley-VCH
- ISBN-10: 3527324291
- ISBN-13: 9783527324293
- Erscheinungsdatum: 28.01.2014
Sprache:
Englisch
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